ArXiv · 2026
Kagome FeSn exhibits an occupied flat band at its terminated surface, whereas bulk FeSn adopts A-type antiferromagnetic order and does not display the same feature. Here, we combine density functional theory with primitive- and doubled-cell analysis and a double-layer tight-binding model to determine how interlayer electronic coupling and magnetic stacking control flat-band formation in FeSn. We identify an occupied Fe-d_(z²)-derived flat-band manifold in the ferromagnetic state that is consistent with the experimentally observed surface feature. Brillouin-zone folding reveals that its flat branch originates from the k_z=π/c sector of the primitive cell, demonstrating that it cannot be understood as an isolated kagome-layer state. Instead, the state depends on coupling between neighboring kagome layers and can be seen as a result of antibonding coupling between nearest neighbor kagome layers. A double-layer tight-binding analysis identifies interlayer Fe-Fe hopping as the dominant microscopic coupling responsible for this behavior, while a contrasting unoccupied flat-band-related manifold is governed primarily by intralayer Fe-Sn hybridization. These results establish interlayer coupling and magnetic stacking as key control parameters for kagome flat bands and highlight how coupling between layers can generate and tune extended correlated-electron states in quantum materials.
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